Giant room-temperature spin caloritronics in spin-semiconducting graphene nanoribbons

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Publication Type pre-print
School or College College of Engineering
Department Materials Science & Engineering
Creator Liu, Feng
Other Author Chen, Xiaobin; Liu, Yizhou; Gu, Bing-Lin; Duan, Wenhui
Title Giant room-temperature spin caloritronics in spin-semiconducting graphene nanoribbons
Date 2014-01-01
Description Spin caloritronics refers to generating spin current by thermal gradient. Here we report a theoretical study demonstrating giant spin caloritronic effects in a new class of materials, called spin semiconductors, which are characterized with a "spin gap," the energy gap between spin-up and -down channels. Generally, spin Seebeck coefficient (Ss ) is shown to increase linearly with the spin gap. Specifically, unprecedented large Ss ∼ 3.4 mV/K and spin figure of merit ZsT ∼ 119 were found in spin-semiconducting graphene nanoribbons (GNRs) with sawtooth (ST) zigzag edges, based on first-principles calculations. Such giant spin caloritronic effects are shown to originate from a large spin gap of ST GNRs, in addition to two other spin-independent features of large band gap and narrow bandwidth which are commonly known for good thermoelectric materials. Our studies suggest that spin-semiconducting nanostructures, such as ST GNRs, are promising candidates for room-temperature spin caloritronics with high efficiency.
Type Text
Publisher American Physical Society
Volume 90
Issue 12
First Page 121403-1
Last Page 121403-5
Language eng
Bibliographic Citation Chen, X., Liu, Y., Gu, B.-L., Duan, W., & Liu, F. (2014). Giant room-temperature spin caloritronics in spin-semiconducting graphene nanoribbons. Physical Review B - Condensed Matter and Materials Physics, 90(12), 121403-1-121403-5.
Rights Management (c) American Physical Society http://dx.doi.org/DOI: 10.1103/PhysRevB.90.121403
Format Medium application/pdf
Format Extent 625,788 bytes
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Reference URL https://collections.lib.utah.edu/ark:/87278/s6bp3bxw